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Michael, this head spaces on the case mouth Sir. Cheers and stay safe!
I'm thinking it probably wouldn't be a good idea. I couldn't find anything definite either way but I messaged Rugers customer service and haven't heard back, they are probably closed by now, but I'll update when I get an answer. Or if you'd like to contact them https://www.ruger.com/footer/contact.html
Ruger response from when I asked them your question. "From what I understand the case on the 9x21 cartridge is longer than the standard 9mm cartridge. I would not use it in the SP101 revolver. For more info, please contact our customer service dept. to speak with a tech. 336-949-5200; M-F; 8-5 ET."